Relation between the High Density Phase and the Very-High Density Phase of Amorphous Solid Water

Details Relation between the High Density Phase and the Very-High Density Phase of Amorphous Solid Water Relation between the High Density Phase and the Very-High Density Phase of Amorphous Solid Water

2004-03-15

arxiv.org/abs/cond-mat/0403365v1

Physics

Condensed Matter

Soft Condensed Matter

5 pages, 4 figs

Scientific paper

10.1103/PhysRevLett.94.107803

It has been suggested that high-density amorphous (HDA) ice is a structurally arrested form of high-density liquid (HDL) water, while low-density amorphous (LDA) ice is a structurally arrested form of low-density liquid (LDL) water. Recent experiments and simulations have been interpreted to support the possibility of a second "distinct" high-density structural state, named very high-density amorphous (VHDA) ice, questioning the LDL-HDL hypothesis. We test this interpretation using extensive computer simulations, and find that VHDA is a more stable form of HDA and that in fact VHDA should be considered as the amorphous ice of the quenched HDL.

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