Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2002-09-06
Europhys. Lett. 60(5), pp. 768-774 (2002)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
Europhysics Letters (in press). 7 pages, including 3 figures
Scientific paper
10.1209/epl/i2002-00374-9
A Landau-Zener multi-crossing method has been used to investigate the tunnel splittings in high quality Mn$_{12}$-acetate single crystals in the pure quantum relaxation regime and for fields applied parallel to the magnetic easy axis. With this method several individual tunneling resonances have been studied over a broad range of time scales. The relaxation is found to be non-exponential and a distribution of tunnel splittings is inferred from the data. The distributions suggest that the inhomogeneity in the tunneling rates is due to disorder that produces a non-zero mean value of the average transverse anisotropy, such as in a solvent disorder model. Further, the effect of intermolecular dipolar interaction on the magnetic relaxation has been studied.
Barco Enrique del
Christou George
Hendrickson David N.
Kent Andrew D.
Rumberger Evan M.
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