Physics – Condensed Matter – Soft Condensed Matter
Scientific paper
2003-10-31
in " Unifying Concepts in Granular Media and Glasses" ed. by A. Coniglio, A. Fierro, H.J. Hermann, M. Nicodemi, 181-194 Elsevi
Physics
Condensed Matter
Soft Condensed Matter
14 pages, 4 figures. To appear in published proceedings of Unifying Concepts in Granular Materials and Glasses, Capri 2003
Scientific paper
We evaluate thermodynamic, geometric and dynamic properties of a short-ranged square well binary mixture to provide a coherent picture of this simple, but rich, model for colloidal interactions. In particular, we compare the location, in the temperature-packing fraction plane, of the geometrical percolation locus, the metastable liquid-gas spinodal and the glass transition lines. Such comparison provides evidence that the gel-state can not be related to the attractive glass transition line directly. Indications are given for the possibility of an indirect link between the two, via an arrested phase separation process. We finally discuss the possibility that a spherical short range attraction may not be sufficient to produce an equilibrium cluster phase at low packing fraction and low temperatures.
Buldyrev Sergey V.
Sciortino Francesco
Tartaglia Piero
Zaccarelli Emanuela
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