Physics – Condensed Matter – Materials Science
Scientific paper
2008-12-23
Phys. Rev. Lett. 103, 037601 (2009)
Physics
Condensed Matter
Materials Science
4 pages,4 figures
Scientific paper
10.1103/PhysRevLett.103.037601
Using a joint approach of density functional theory and model calculations, we demonstrate that a prototypical charge ordered half-doped manganite, La$_{1/2}$Ca$_{1/2}$MnO$_3$ is multiferroic. The combination of a peculiar charge-orbital ordering and a tendency to form spin dimers breaks inversion symmetry, leads to a ferroelectric ground-state with a polarization up to several $\mu C/cm^2$. The presence of improper ferroelectricity does not depend on hotly debated structural details of this material: in the Zener-polaron structure we find a similar dramatic ferroelectric response with a large polarization of purely magnetic origin.
Giovannetti Gianluca
Kumar Sanjeev
Picozzi Silvia
van den Brink Jeroen
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