Physics – Condensed Matter – Materials Science
Scientific paper
2003-03-17
Physics
Condensed Matter
Materials Science
8 pages, 7 figures
Scientific paper
10.1103/PhysRevB.68.134439
A detailed investigation of mesoscopic magnetic and crystallographic phase separation in Ca(1-x)La(x)MnO3, 0.00<=x<=0.20, is reported. Neutron powder diffraction and DC-magnetization techniques have been used to isolate the different roles played by electrons doped into the eg level as a function of their concentration x. The presence of multiple low-temperature magnetic and crystallographic phases within individual polycrystalline samples is argued to be an intrinsic feature of the system that follows from the shifting balance between competing FM and AFM interactions as a function of temperature. FM double-exchange interactions associated with doped eg electrons are favored over competing AFM interactions at higher temperatures, and couple more strongly with the lattice via orbital polarization. These FM interactions thereby play a privileged role, even at low eg electron concentrations, by virtue of structural modifications induced above the AFM transition temperatures.
Argyriou Dimitri N.
Granado Eduardo
Ling Chris D.
Lynn Jacob W.
Neumeier John J.
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