Physics – Condensed Matter – Statistical Mechanics
Scientific paper
2003-01-16
Proc. Natl. Acad. Sci. USA 100, 9710 (2003)
Physics
Condensed Matter
Statistical Mechanics
5 pages, 5 figures
Scientific paper
10.1073/pnas.1233719100
We introduce a coarse-grained model for atomic glass formers. Its elements are physically motivated local microscopic dynamical rules parameterized by observables. Results of the model are established and used to interpret the measured behaviors of supercooled fluids approaching glass transitions. The model predicts the presence of a crossover from hierarchical super-Arrhenius dynamics at short length scales to diffusive Arrhenius dynamics at large length scales. This prediction distinguishes our model from other theories of glass formers and can be tested by experiment.
Chandler David
Garrahan Juan P.
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