Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2010-12-07
Nature Materials 9, 550-554 (2010)
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
Scientific paper
10.1038/nmat2768
In a zero-dimensional superconductor, quantum size effects(QSE) not only set the limit to superconductivity, but are also at the heart of new phenomena such as shell effects, which have been predicted to result in large enhancements of the superconducting energy gap. Here, we experimentally demonstrate these QSE through measurements on single, isolated Pb and Sn nanoparticles. In both systems superconductivity is ultimately quenched at sizes governed by the dominance of the quantum fluctuations of the order parameter. However, before the destruction of superconductivity, in Sn nanoparticles we observe giant oscillations in the superconducting energy gap with particle size leading to enhancements as large as 60%. These oscillations are the first experimental proof of coherent shell effects in nanoscale superconductors. Contrarily, we observe no such oscillations in the gap for Pb nanoparticles, which is ascribed to the suppression of shell effects for shorter coherence lengths. Our study paves the way to exploit QSE in boosting superconductivity in low-dimensional systems.
Bose Sangita
Brihuega Ivan
Garcia-Garcia Antonio M.
Kern Klaus
Michaelis Christian H.
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