Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2010-11-30
Phys. Rev. B 83, 014401 (2011)
Physics
Condensed Matter
Strongly Correlated Electrons
6 pages, 8 figures
Scientific paper
10.1103/PhysRevB.83.014401
We report the remarkably robust ferroelectric state in the multiferroic compound Mn$_{1-x}$Zn$_x$WO$_4$. The substitution of the magnetic Mn$^{2+}$ with nonmagnetic Zn$^{2+}$ reduces the magnetic exchange and provides control of the various magnetic and multiferroic states of MnWO$_4$. Only 5 % of Zn substitution results in a complete suppression of the frustrated collinear (paraelectric) low temperature phase. The helical magnetic and ferroelectric phase develops as the ground state. The multiferroic state is stable up to a high level of substitution of more than 50 %. The magnetic, thermodynamic, and dielectric properties as well as the ferroelectric polarization of single crystals of Mn$_{1-x}$Zn$_x$WO$_4$ are studied for different substitutions up to x=0.5. The magnetic phases have been identified in single crystal neutron scattering experiments. The ferroelectric polarization scales with the neutron intensity of the incommensurate peak of the helical phase.
Chaudhury Rajit P.
Chu Cheng-Wei
Fernandez-Baca Jaime A.
Lorenz Beat
Mook Herbert A.
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