Classical and quantum magnetization reversal studied in nanometer-sized particles and clusters

Physics – Condensed Matter – Mesoscale and Nanoscale Physics

Scientific paper

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94 pages, 59 figures, extracted from Habilitation of W. Wernsdorfer, April 2001

Scientific paper

Nanometer-sized magnetic particles have generated continuous interest as the study of their properties has proved to be scientifically and technologically very challenging. In this article we reviewed the most important theories and experimental results concerning the magnetization reversal of single-domain particles,clusters and molecular clusters. Sect.1 reviews briefly the commonly used measuring techniques. Among them, electrical transport measurements, Hall probes and micro-SQUID techniques seem to be the most convenient techniques for low temperature measurements. Sect.2 discusses the mechanisms of magnetization reversal in single domain particles at zero Kelvin. The influence of temperature on the magnetization reversal is reported in Sect.3. Finally, Sect.4 shows that for very small systems or very low temperature, magnetization can reverse via quantum tunneling. The boundary between classical and quantum physics has become a very attractive field of research. This section discusses detailed measurements which demonstrated that molecular magnets offer an unique opportunity to explore the quantum dynamics of a large but finite spin. We then discussed tunneling in nanoparticles and showed how one might give a definite proof of their quantum character at low temperature.

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