Fluid-solid phase-separation in hard-sphere mixtures is unrelated to bond-percolation

Details Fluid-solid phase-separation in hard-sphere mixtures is unrelated to bond-percolation Fluid-solid phase-separation in hard-sphere mixtures is unrelated to bond-percolation

2000-01-18

arxiv.org/abs/cond-mat/0001241v1

Phys. Rev. Lett. 84, 1840 (2000)

Physics

Condensed Matter

Soft Condensed Matter

Comment, 1 page, to appear in Phys. Rev. Lett

Scientific paper

10.1103/PhysRevLett.84.1840

In a recent letter, Buhot proposes that entropy driven phase-separation in hard-core binary mixtures is directly related to a bond-percolation transition. However, at least for binary hard-sphere mixtures, calculations based on an accurate approximation to g_{ll}(r) demonstrate that n_b varies widely along the phase-boundaries calculated directly by simulations, implying that bond-percolation is unrelated to the phase-separation in these systems.

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