Size dependent tunneling and optical spectroscopy of CdSe quantum rods

Physics – Condensed Matter – Mesoscale and Nanoscale Physics

Scientific paper

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Accepted to PRL (nearly final version). 4 pages in revtex, 4 figures

Scientific paper

10.1103/PhysRevLett.89.086801

Photoluminescence excitation spectroscopy and scanning tunneling spectroscopy are used to study the electronic states in CdSe quantum rods that manifest a transition from a zero dimensional to a one dimensional quantum confined structure. Both optical and tunneling spectra show that the level structure depends primarily on the rod diameter and not on length. With increasing diameter, the band-gap and the excited state level spacings shift to the red. The level structure was assigned using a multi-band effective-mass model, showing a similar dependence on rod dimensions.

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