Potentiodynamic Electrochemical Impedance Spectroscopy of Silver on Platinum in Underpotential and Overpotential Deposition

Details Potentiodynamic Electrochemical Impedance Spectroscopy of Silver on Platinum in Underpotential and Overpotential Deposition Potentiodynamic Electrochemical Impedance Spectroscopy of Silver on Platinum in Underpotential and Overpotential Deposition

2003-10-20

arxiv.org/abs/cond-mat/0310449v1

Surf. Sci. 566-568 (2004) 315

Physics

Condensed Matter

Materials Science

submitted to Surface Science

Scientific paper

10.1016/j.susc.2004.05.061

Simultaneous monitoring of ac and dc responses of the electrode-electrolyte interface with potentiodynamic electrochemical impedance spectroscopy (PDEIS) in silver underpotential and overpotential deposition on platinum has confirmed the role of intrinsic Pt surface changes in the irreversibility of Ag underpotential deposition and disclosed exceptionally high stability of Ag monolayer on Pt. PDEIS has been demonstrated to be a convenient means for wet surface chemistry monitoring.

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