Thermodynamics of binary mixture glasses

Details Thermodynamics of binary mixture glasses Thermodynamics of binary mixture glasses

1999-03-08

arxiv.org/abs/cond-mat/9903129v2

J.Chem.Phys. n.111, 9039 (1999)

Physics

Condensed Matter

28 pages, 8 figures, revised version, accepted for the publication in the Journal of Chemical Physics

Scientific paper

10.1063/1.480246

We compute the thermodynamic properties of the glass phase in a binary mixture of soft spheres. Our approach is a generalization to mixtures of the replica strategy, recently proposed by Mezard and Parisi, providing a first principle statistical mechanics computation of the thermodynamics of glasses. The method starts from the inter-atomic potentials, and translates the problem into the study of a molecular liquid. We compare uor analytical predictions to numerical simulations, focusing onto the values of the thermodynamic transition and the configurational entropy.

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