Structure, rotational dynamics, and superfluidity of small OCS-doped He clusters

Details Structure, rotational dynamics, and superfluidity of small OCS-doped He clusters Structure, rotational dynamics, and superfluidity of small OCS-doped He clusters

2002-12-12

arxiv.org/abs/cond-mat/0212266v1

Physics

Condensed Matter

4 pages. TeX (requires revtex4) + 3 ps figures (1 color)

Scientific paper

10.1103/PhysRevLett.90.143401

The structural and dynamical properties of OCS molecules solvated in Helium clusters are studied using reptation quantum Monte Carlo, for cluster sizes n=3-20 He atoms. Computer simulations allow us to establish a relation between the rotational spectrum of the solvated molecule and the structure of the He solvent, and of both with the onset of superfluidity. Our results agree with a recent spectroscopic study of this system, and provide a more complex and detailed microscopic picture of this system than inferred from experiments.

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