Charge ordering and chemical potential shift in La$_{2-x}$Sr$_x$NiO$_4$ studied by photoemission spectroscopy

Details Charge ordering and chemical potential shift in La$_{2-x}$Sr$_x$NiO$_4$ studied by photoemission spectroscopy Charge ordering and chemical potential shift in La$_{2-x}$Sr$_x$NiO$_4$ studied by photoemission spectroscopy

1999-08-02

arxiv.org/abs/cond-mat/9908014v1

Physics

Condensed Matter

Strongly Correlated Electrons

5 pages, 4 figures

Scientific paper

10.1103/PhysRevB.61.15515

We have studied the chemical potential shift in La$_{2-x}$Sr$_x$NiO$_4$ and the charge ordering transition in La$_{1.67}$Sr$_{0.33}$NiO$_4$ by photoemission spectroscopy. The result shows a large ($\sim$ 1 eV/hole) downward shift of the chemical potential with hole doping in the high-doping regime ($\delta \gtrsim$ 0.33) while the shift is suppressed in the low-doping regime ($\delta \lesssim$ 0.33). This suppression is attributed to a segregation of doped holes on a microscopic scale when the hole concentration is lower than $\delta \simeq 1/3$. In the $\delta = 1/3$ sample, the photoemission intensity at the chemical potential vanishes below the charge ordering transition temperature $T_{\rm CO}=$ 240 K.

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