Two inequivalent sublattices and orbital ordering in MnV2O4 studied by 51V NMR

Physics – Condensed Matter – Strongly Correlated Electrons

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4 pages, 4 figures, title changed, published in PRB as a rapid comm

Scientific paper

10.1103/PhysRevB.80.140406

We report detailed 51V NMR spectra in a single crystal of MnV2O4. The vanadium spectrum reveals two peaks in the orbitally ordered state, which arise from different internal hyperfine fields at two different V sublattices. These internal fields evolve smoothly with externally applied field, and show no change in structure that would suggest a change of the orbital ordering. The result is consistent with the orbital ordering model recently proposed by Sarkar et al. [Phys. Rev. Lett. 102, 216405 (2009)] in which the same orbital that is a mixture of t_2g orbitals rotates by about 45$^\circ$ alternately within and between orbital chains in the I4_1/a tetragonal space group.

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