Evolution of a Metal to Insulator Transition in Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_{2}$, as seen by ARPES

Physics – Condensed Matter – Strongly Correlated Electrons

Scientific paper

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10 pages, 12 figures, accepted by PRB; a high quality pdf is available at http://helios.physics.utoronto.ca/~fronning/Ronnin

Scientific paper

10.1103/PhysRevB.67.165101

We present angle resolved photoemission (ARPES) data on Na-doped Ca$_2$CuO$_2$Cl$_2$. We demonstrate that the chemical potential shifts upon doping the system across the insulator to metal transition. The resulting low energy spectra reveal a gap structure which appears to deviate from the canonical $d_{x2-y2} ~ |cos(k_x a)-cos(k_y a)|$ form. To reconcile the measured gap structure with d-wave superconductivity one can understand the data in terms of two gaps, a very small one contributing to the nodal region and a very large one dominating the anti-nodal region. The latter is a result of the electronic structure observed in the undoped antiferromagnetic insulator. Furthermore, the low energy electronic structure of the metallic sample contains a two component structure in the nodal direction, and a change in velocity of the dispersion in the nodal direction at roughly 50 meV. We discuss these results in connection with photoemission data on other cuprate systems.

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