Physics – Condensed Matter – Mesoscale and Nanoscale Physics
Scientific paper
2009-06-29
Phys. Rev. Lett. 104, 066804 (2010) - Published February 12, 2010
Physics
Condensed Matter
Mesoscale and Nanoscale Physics
5 pages, 3 figures, submitted to Phys. Rev. Lett
Scientific paper
We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically "forbidden" transitions. This process corresponds to one-to-one conversion of a photon absorbed by the dot into a polarized nuclear spin, which also has potential for initialization of hole spin in QDs. Pumping via the "forbidden" transition is a manifestation of the "optical solid effect", an optical analogue of the effect previously observed in electron spin resonance experiments in the solid state. We find that by employing this effect, nuclear polarization of 65% can be achieved, the highest reported so far in optical orientation studies in QDs. The efficiency of the spin pumping exceeds that employing the allowed transition, which saturates due to the low probability of electron-nuclear spin flip-flop.
Chekhovich E. A.
Kavokin K. V.
Krysa Andrey B.
Makhonin M. N.
Skolnick Maurice S.
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