Physics – Condensed Matter – Strongly Correlated Electrons
Scientific paper
2001-03-14
Phys. Rev. Lett. 86, 3879 (2001)
Physics
Condensed Matter
Strongly Correlated Electrons
4 pages, 3 figures, to appear in Phys. Rev. Lett
Scientific paper
10.1103/PhysRevLett.86.3879
We investigate the highly frustrated spin and orbital superexchange interactions in cubic vanadates. The fluctuations of $t_{2g}$ orbitals trigger a {\it novel mechanism of ferromagnetic interactions} between spins S=1 of V$^{3+}$ ions along one of the cubic directions which operates already in the absence of Hund's rule exchange $J_H$, and leads to the C-type antiferromagnetic phase in LaVO$_3$. The Jahn-Teller effect can stabilize the orbital ordering and the G-type antiferromagnetic phase at low temperatures, but large entropy due to orbital fluctuations favors again the C-phase at higher temperatures, as observed in YVO$_3$.
Horsch Peter
Khaliullin Giniyat
Oles' Andrzej M.
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