Physics – Condensed Matter – Soft Condensed Matter
Scientific paper
2007-08-22
Physics
Condensed Matter
Soft Condensed Matter
Version 2. Major changes. New data
Scientific paper
10.1103/PhysRevLett.100.126001
We discuss simulations of a simple model for polymer blends in the framework of the Rouse model. At odds with standard predictions, large dynamic asymmetry between the two components induces strong non-exponentiality of the Rouse modes for the fast component. Despite chains being much shorter than the entanglement length, it also induces dynamic features resembling a crossover to entangled-like chain dynamics. This unusual behavior is associated to strong memory effects which break down the assumption of time uncorrelation of the external forces acting on the tagged chain.
Colmenero Juan
Moreno Angel J.
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