Light scattering spectra of supercooled molecular liquids

Details Light scattering spectra of supercooled molecular liquids Light scattering spectra of supercooled molecular liquids

2000-06-13

arxiv.org/abs/cond-mat/0006214v1

Phys. Rev. E 63, 061209 (2001)

Physics

Condensed Matter

Statistical Mechanics

12 pages

Scientific paper

10.1103/PhysRevE.63.061209

The light scattering spectra of molecular liquids are derived within a generalized hydrodynamics. The wave vector and scattering angle dependences are given in the most general case and the change of the spectral features from liquid to solidlike is discussed without phenomenological model assumptions for (general) dielectric systems without long-ranged order. Exact microscopic expressions are derived for the frequency-dependent transport kernels, generalized thermodynamic derivatives and the background spectra.

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