First complete isotopic analysis of Solar Wind heavy noble gases in Genesis Aluminum collectors

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[6200] Planetary Sciences: Solar System Objects

Scientific paper

Analyses of noble gases implanted into Genesis Solar Wind (SW) collectors and their comparison with the gases from solar-wind rich lunar and meteoritic materials may constrain an extent of temporal variations of isotopic composition of the solar wind. Here we report our isotope measurements of all heavy noble gas isotopes including low abundant 126Xe, 124Xe and 78Kr. Two aluminum Genesis collectors were used in this study: Aluminum on Sapphire (AloS) and Polished Aluminum Collector (PAC). Solar Wind (SW) noble gases were extracted using IR- and UV-lasers operated in Q-switched mode. Purified gases were analyzed in the modified 8-multiplier mass spectrometer Noblesse, custom built by Nu-Instruments (UK) for microanalyses of heavy noble gases. SW-Ar was analyzed using UV-depth profiling, which clearly demonstrated depth dependant isotope fractionation caused by SW-implantation at constant ion velocities. The cumulative SW-Ar composition is in good agreement with our earlier analyses made by a single multiplier mass spectrometer (36Ar/38Ar = 5.501 ± 0.002, [1]). SW-Kr was found to have the following isotopic composition: 86Kr/84Kr = .3012 ± .0004, 83Kr/84Kr = .2034 ± .0002, 82Kr/84Kr = .2054 ± .0002, 80Kr/84Kr = .0412 ± .0002, and 78Kr/84Kr = .00642 ± .00005. These results are statistically indistinguishable from SW-Kr composition based on the lunar regolith data [2]. Our best current estimate of SW-Xe composition obtained from 25 independent analyses ran at different experimental conditions is: 136Xe/132Xe = .3003 ± .0006, 134Xe/132Xe = .3692 ± .0007, 131Xe/132Xe = .8263 ± .0013, 130Xe/132Xe = .1649 ± .0004, 129Xe/132Xe = 1.0401 ± .00010, 128Xe/132Xe = .0842 ± .0003, 126Xe/132Xe = .00417 ± .00009, and 124Xe/132Xe = .00492 ± .00007. Although small systematical difference between these numbers and lunar SW-Xe is observed, more accurate SW-Xe lunar regolith measurements are required to understand whether or not these differences are real. The total amounts of heavy noble gases accumulated over 853 days of collection are: (2.81 ± .19)E+10, (1.08 ± .05)E+07, and (1.15 ± .04)E+06 atoms/cm2 of 36Ar, 84Kr and 132Xe correspondently. This work is supported by NASA grant NNX07AM76G. [1] Meshik A. P. et al. Science 318, 2007, [2] Pepin R. O. et al. 1995. GCA 59.

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