Vibrational excitation of diatomic molecular ions in strong-field ionization of diatomic molecules

Details Vibrational excitation of diatomic molecular ions in strong-field ionization of diatomic molecules Vibrational excitation of diatomic molecular ions in strong-field ionization of diatomic molecules

2005-01-31

arxiv.org/abs/physics/0501157v2

Phys. Rev. Lett. 95, 073004 (2005)

Physics

Atomic Physics

4 pages, 4 figures

Scientific paper

10.1103/PhysRevLett.95.073004

A model based on the strong-field and Born-Oppenheimer approximations qualitatively describes the distribution over vibrational states formed in a diatomic molecular ion following ionization of the neutral molecule by intense laser pulses. Good agreement is found with a recent experiment [X. Urbain et al., Phys. Rev. Lett. 92, 163004 (2004)]. In particular, the observed deviation from a Franck-Condon-like distribution is reproduced. Additionally, we demonstrate control of the vibrational distribution by a variation of the peak intensity or a change of frequency of the laser pulse.

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