Interplay of creation, propagation, and relaxation of an excitation in a dimer

Details Interplay of creation, propagation, and relaxation of an excitation in a dimer Interplay of creation, propagation, and relaxation of an excitation in a dimer

1999-01-06

arxiv.org/abs/quant-ph/9901007v1

Chem.Phys. 236 (1998) 157-179

Physics

Quantum Physics

LATEX, 19 pages, 16 PostScript figures

Scientific paper

Interplay of simultaneous creation, annihilation, propagation, and relaxation of an excitation in molecular condensates interacting with an ultrashort quantum optical pulse is studied in general and specialized to a dimer. A microscopic model appropriate for such systems (with strong exciton-phonon coupling) is presented. It also incorporates effects of (quantum) noise in the optical field. A variety of new features in the initial stage of excitation dynamics (when it is being created) is revealed; a strong influence of the coherent excitation propagation on the processes of excitation creation and annihilation in a molecule strongly interacting with phonons is the most remarkable one.

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