Spectral properties of molecular oligomers. A non-Markovian quantum state diffusion approach

Details Spectral properties of molecular oligomers. A non-Markovian quantum state diffusion approach Spectral properties of molecular oligomers. A non-Markovian quantum state diffusion approach

2010-08-21

arxiv.org/abs/1008.3611v1

International Journal of Modern Physics B (IJMPB), 24, 5060 (2010)

Physics

Chemical Physics

Scientific paper

10.1142/S0217979210057201

Absorption spectra of small molecular aggregates (oligomers) are considered. The dipole-dipole interaction between the monomers leads to shifts of the oligomer spectra with respect to the monomer absorption. The line-shapes of monomer as well as oligomer absorption depend strongly on the coupling to vibrational modes. Using a recently developed approach [Roden et. al, PRL 103, 058301] we investigate the length dependence of spectra of one-dimensional aggregates for various values of the interaction strength between the monomers. It is demonstrated, that the present approach is well suited to describe the occurrence of the J- and H-bands.

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