Distribution of 127I and 129I in precipitation at high European latitudes

Physics

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Atmospheric Processes: Precipitation (1854), Hydrology: Human Impacts, Hydrology: Anthropogenic Effects (4802, 4902), Geochemistry: Radiogenic Isotope Geochemistry, Geochemistry: Composition Of The Hydrosphere

Scientific paper

We here present the most extensive data set on the distribution of 127I and 129I in precipitation (rain and snow) covering the period 2000-2006 and European latitudes 55°N-68°N. Our results indicate a wide variation in the concentrations and fluxes of the two isotopes associated with generally higher values at near coastal sites compared to the inland ones. Total wet-related annual deposition of 127I and 129I on Sweden and Denmark is estimated at about 1.2 × 109 g and 60 g respectively. The average annual 129I wet deposition accounts for <1% and <0.05% of the total annual gaseous and liquid, respectively, discharges from the Sellafiled and La Hague Facilities. The 127I annual wet deposition represents <1% of the estimated global oceanic iodine flux. Air mass trajectories suggest that events of enhanced 129I in precipitation are closely related to southwesterly weather fronts from regions of elevated concentrations.

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