Physics
Scientific paper
Oct 2008
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2008georl..3519807x&link_type=abstract
Geophysical Research Letters, Volume 35, Issue 19, CiteID L19807
Physics
Atmospheric Composition And Structure: Pollution: Urban And Regional (0305, 0478, 4251), Atmospheric Composition And Structure: Constituent Sources And Sinks, Atmospheric Composition And Structure: Middle Atmosphere: Constituent Transport And Chemistry (3334)
Scientific paper
Many mountainous regions in South China have been confronted with the consequences of acidic deposition, but studies on atmospheric S sources are still very limited. In this study, isotopic ratios in mosses were used to discriminate atmospheric S sources. A continuous increase in S isotopic ratios was observed from the south to the north in mountainous mosses and in accord with the previously reported changing trends in urban mosses, indicating a contribution of local anthropogenic S from urban cities. Based on comparisons of S isotopic ratios in mountainous mosses with those in nearby urban mosses, we found that mountainous mosses had significantly higher 34S contents than urban mosses, especially in West China, reflecting an introduction of 34S-enriched sulphur. In conjunction with cloud water data in the literature, we concluded that 34S-enriched sulphur in northerly air masses contributed much to atmospheric S in southern Chinese mountainous areas.
Liu Cong-Qiang
Liu Xue-Yan
Tang Cong-Guo
Xiao Hong-Wei
Xiao Hua-Yun
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