Physics
Scientific paper
Apr 1978
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1978georl...5..317a&link_type=abstract
Geophysical Research Letters, vol. 5, Apr. 1978, p. 317-320.
Physics
7
Atmospheric Attenuation, Heterodyning, Infrared Spectrometers, Ozonometry, Stratosphere, Absorption Spectra, Air Pollution, Atmospheric Composition, Carbon Dioxide Lasers, Line Spectra, Vertical Distribution
Scientific paper
Measurements of a stratospheric ozone concentration profile are made by detecting infrared absorption lines with a heterodyne spectrometer. The infrared spectrometer is based on a line-by-line tunable CO2 lasers, a liquid-nitrogen cooled HgCdTe photomixer, and a 64-channel spectral line receiver. The infrared radiation from the source is mixed with local-oscillator radiation. The difference frequency signal in a bandwidth above and below the local-oscillator frequency is detected. The intensity in each sideband is found by subtracting sideband contributions. It is found that absolute total column density is 0.32 plus or minus 0.02 cm-atm with a peak mixing ratio at about 24 km. The (7,1,6)-(7,1,7) O3 line center frequency is identified as 1043.1772/cm. Future work will involve a number of ozone absorption lines and measurements of diurnal variation. Completely resolved stratospheric lines may be inverted to yield concentration profiles of trace constituents and stratospheric gases.
Abbas Merza
Brown Warren L.
Buhl David
Kostiuk Theodor,
Kunde Virgil G.
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