Vibrational States of the Hydrogen Isotopes on Pd(111)

Details Vibrational States of the Hydrogen Isotopes on Pd(111) Vibrational States of the Hydrogen Isotopes on Pd(111)

1994-03-16

arxiv.org/abs/chem-ph/9403008v1

Physics

Chemical Physics

Surface Science Letters, 302, L305 (1994)

Scientific paper

10.1016/0039-6028(94)90826-5

The ground and excited vibrational states for the three hydrogen isotopes on the Pd(111) surface have been calculated. Notable features of these states are the high degree of anharmonicity, which is most prominently seen in the weak isotopic dependence of the parallel vibrational transition, and the narrow bandwidths of these states, which imply that atomic hydrogen is localized on a particular surface site on time scales of 100 picoseconds or more. Experiments to resolve ambiguities concerning the present system are suggested.

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