Vector Correlation in the Photodissociation of Metal Nitrosyls

Details Vector Correlation in the Photodissociation of Metal Nitrosyls Vector Correlation in the Photodissociation of Metal Nitrosyls

Jun 2010

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2010mss..conferg08b&link_type=abstract

"International Symposium On Molecular Spectroscopy, 65th Meeting, Held 21-25 June, 2010 at Ohio State University. http://molspec

Physics

Mini-Symposium: Metal Containing Molecules

Scientific paper

The vector correlation in the photodissociation of metal nitrosyls has been determined using linearly-polarized laser light and velocity-mapped ion imaging. The 225-nm dissociation beam excites a doubly-degenerate metal-to-ligand charge transfer in both eta5-C5H5NiNO and Co(CO)3NO. State-resolved detection of the NO product through the A (v'=0) ← X (v"=0) transition reveals that both molecules dissociate promptly with a high degree of vector correlation.

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