Physics
Scientific paper
Dec 1994
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1994e%26psl.128..653r&link_type=abstract
Earth and Planetary Science Letters (ISSN 0012-821X), vol. 128, no. 3-4, p. 653-670
Physics
9
Geochronology, Nuclear Fission, Uranium, Xenon, Lead (Metal), Thorium Isotopes
Scientific paper
U-Xe chronology requires knowledge of the product of the decay constant (lambdasf) and the fractional yield of Xe-136 (Ysf-136) produced by the spontaneous fissin of U-238. However, values derived from U oxides are in conflict with those obtained from U-bearing accessory minerals. We present combined U-Pb and U-Xe data for carefully selected suite of zircon and monazite separates. All samples have precise, concordant or near-concordant U-Pb ages and yield a lambdasf* Ysf-136 value of (6.38 +/- 0.18) x 10-18/a. Recoil loss of fissiongenic Xe was corrected for numerically or circumvented by abrading samples or analyzing very large crystals. Old crystal cores that might have retained their fission Xe but not their radiogenic Pb were not detected in any of the samples. No significant contribution of Xe from Th-232 fission is expected as long as the Th/U ratio is less than or = 10. Taken together, these observations indicate that the derived value for lambdasf* Ysf-136 is correct. This value is similar to that from earlier studies of accessory minerals, but some 20% higher than that determined recently from carefully selected U minerals, including pitchblende, uraninite and coffinite. This suggests that U oxides systematically lose fissiogenic Xe, possibly due to regeneration of the crystal lattice or changes in oxidation state. U-Xe from such minerals should be interpreted with caution.
Hebeda Erhard H.
Ragettli Riccarda A.
Signer Peter
Wieler Rainer
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