Physics
Scientific paper
Jul 1982
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1982stan.reptq....b&link_type=abstract
Final Technical Report, 1 Jan. 1980 - 30 Jun. 1982 Stanford Univ., CA. Lab. of Physics.
Physics
Atmospheric Composition, Expansion, Molecular Beams, Planetary Atmospheres, Raman Spectroscopy, Supercooling, Clumps, Electron Transitions, High Resolution, Pulsed Radiation, Steady State, Supersonic Speed, Transit Time
Scientific paper
The measurement of high resolution pulsed and continuous wave (CW) coherent anti-Stokes Raman spectroscopy (CARS) measurements in pulsed and steady state supersonic expansions were demonstrated. Pulsed molecular beam sources were characterized, and saturation of a Raman transition and, for the first time, the Raman spectrum of a complex molecular cluster were observed. The observation of CW CARS spectra in a molecular expansion and the effects of transit time broadening is described. Supersonic expansion is established as a viable technique for high resolution Raman spectroscopy of cold molecules with resolutions of 100 MH2.
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