Two-photon ionization of Helium studied with the multiconfigurational time-dependent Hartree-Fock method

Details Two-photon ionization of Helium studied with the multiconfigurational time-dependent Hartree-Fock method Two-photon ionization of Helium studied with the multiconfigurational time-dependent Hartree-Fock method

2010-10-26

arxiv.org/abs/1010.5422v1

Journal of Chemical Physics 134, issue 8, 084106 (2011)

Physics

Atomic Physics

Scientific paper

10.1063/1.3553176

The multiconfigurational time-dependent Hartree-Fock method (MCTDHF) is applied for simulations of the two-photon ionization of Helium. We present results for the single- and double ionization from the groundstate for photon energies in the non-sequential regime, and compare them to direct solutions of the Schr\"odinger equation using the time-dependent (full) Configuration Interaction method (TDCI). We find that the single-ionization is accurately reproduced by MCTDHF, whereas the double ionization results correctly capture the main trends of TDCI.

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