Two-Dimensional (2+n) Rempi Spectroscopy: State Interactions, Photofragmentations and Energetics of the Hydrogen Halides

Details Two-Dimensional (2+n) Rempi Spectroscopy: State Interactions, Photofragmentations and Energetics of the Hydrogen Halides Two-Dimensional (2+n) Rempi Spectroscopy: State Interactions, Photofragmentations and Energetics of the Hydrogen Halides

Jun 2011

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2011mss..confemf08l&link_type=abstract

"International Symposium On Molecular Spectroscopy, 66th Meeting, Held 20-24 June, 2011 at Ohio State University. http://molspec

Physics

Electronic

Scientific paper

Mass spectra are recorded for one-colour (2 + n) resonance enhanced multiphoton ionization (REMPI) of HX (X = Cl, Br) as a function of resonance excitation energy to obtain two-dimensional REMPI data. Perturbations due to Rydberg to ion-pair state interactions show as line shifts, ion signal intensity variations as well as band width broadenings depending on rotational quantum numbers, J ' . The data allow determination of parameters relevant to the nature and strength of state interactions as well as dissociation and ionization processes. Alterations in X+ and HX+ signal intensities prove to be very useful for spectra assignments.
Agust Kvaran, Kristjan Matthiasson and Huasheng Wang, " Two-Dimensional (2+n) Resonance Enhanced Multiphoton Ionization of HCl: State Interactions and Photorupture Channels via Low-Energy Triplet Rydberg States ", J. Chem. Phys., 131(4), 044324, (2009).

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