Towards time resolved core level photoelectron spectroscopy with femtosecond x-ray free-electron lasers

Details Towards time resolved core level photoelectron spectroscopy with femtosecond x-ray free-electron lasers Towards time resolved core level photoelectron spectroscopy with femtosecond x-ray free-electron lasers

Mar 2008

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2008njph...10c3004p&link_type=abstract

New Journal of Physics, Volume 10, Issue 3, pp. 033004 (2008).

Physics

17

Scientific paper

We have performed core level photoelectron spectroscopy on a W(110) single crystal with femtosecond XUV pulses from the free-electron laser at Hamburg (FLASH). We demonstrate experimentally and through theoretical modelling that for a suitable range of photon fluences per pulse, time-resolved photoemission experiments on solid surfaces are possible. Using FLASH pulses in combination with a synchronized optical laser, we have performed femtosecond time-resolved core-level photoelectron spectroscopy and observed sideband formation on the W 4f lines indicating a cross correlation between femtosecond optical and XUV pulses.

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