Thermodynamics of aqueous uranyl ion: Apparent and partial molar heat capacities and volumes of aqueous uranyl perchlorate from 10 to 55°C

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Apparent molar heat capacities and volumes of aqueous solutions containing UO 2 (ClO 4 ) 2 in dilute ( 0.06 molal) HClO 4 have been determined from 10 to 55°C. These results have been analyzed using Young's rule to obtain apparent molar volumes and heat capacities for the solute UO 2 (ClO 4 2 ). The temperature dependences of the conventional standard-state heat capacity and volume functions for UO 2 2+ (aq) are well represented by the following equations: that are valid from 10 to 55°C. These results differ substantially from results of earlier measurements employing different uranyl salts. These differences are likely due to the presence of ion-paired or hydrolyzed U (VI) species in the earlier studies.

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