Theory of selective excitation in Stimulated Raman Scattering

Details Theory of selective excitation in Stimulated Raman Scattering Theory of selective excitation in Stimulated Raman Scattering

2003-06-24

arxiv.org/abs/physics/0306166v2

Physics

Chemical Physics

RevTeX4,10 pages, 5 figures, submitted to Phys.Rev.A

Scientific paper

10.1103/PhysRevA.69.013801

A semiclassical model is used to investigate the possibility of selectively exciting one of two closely spaced, uncoupled Raman transitions. The duration of the intense pump pulse that creates the Raman coherence is shorter than the vibrational period of a molecule (impulsive regime of interaction). Pulse shapes are found that provide either enhancement or suppression of particular vibrational excitations.

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