The pressure dependence of the reaction between ClO and OClO at 226 K

Details The pressure dependence of the reaction between ClO and OClO at 226 K The pressure dependence of the reaction between ClO and OClO at 226 K

Dec 1990

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=1990georl..17.2357p&link_type=abstract

Geophysical Research Letters (ISSN 0094-8276), vol. 17, Dec. 1990, p. 2357-2360. Research supported by the Chemical Manufacturer

Physics

5

Atmospheric Chemistry, Chemical Reactions, Chlorine Oxides, Ozone Depletion, Reaction Kinetics, Stratosphere, Antarctic Regions, Photolysis, Pressure Dependence, Spectroscopy, Temperature Dependence, Ultraviolet Absorption

Scientific paper

The first study of the gas-phase kinetics of the reaction between ClO and OClO to form Cl2O3 is reported. The reaction has a strong pressure dependence and the thermolecular rate constant at 226 K is (2.8 + or - 2.2) x 10 to the -31st cm exp 6/molecule exp 2/s. The importance of the reaction for Antarctic ozone depletion is discussed, and an explanation is offered for the unexpected behavior observed in earlier studies of the OClO/NO2 system.

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