Studies on optimizing potential energy functions for maximal intrinsic hyperpolarizability

Details Studies on optimizing potential energy functions for maximal intrinsic hyperpolarizability Studies on optimizing potential energy functions for maximal intrinsic hyperpolarizability

2007-04-13

arxiv.org/abs/0704.1687v1

Physics

Optics

9 pages, 9 figures

Scientific paper

10.1103/PhysRevA.76.053831

We use numerical optimization to study the properties of (1) the class of one-dimensional potential energy functions and (2) systems of point charges in two-dimensions that yield the largest hyperpolarizabilities, which we find to be within 30% of the fundamental limit. We investigate the character of the potential energy functions and resulting wavefunctions and find that a broad range of potentials yield the same intrinsic hyperpolarizability ceiling of 0.709.

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