Steering a molecule into dissociation via vibrational excitation

Details Steering a molecule into dissociation via vibrational excitation Steering a molecule into dissociation via vibrational excitation

Aug 2009

adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2009njph...11h3014k&link_type=abstract

New Journal of Physics, Volume 11, Issue 8, pp. 083014 (2009).

Physics

4

Scientific paper

For a laser driven molecule, we show that the ionization and the dissociation channels can be separated by preparing the molecule in a specific vibrational state. Specifically, we investigate the dynamics of the hydrogen molecular ion under a femtosecond infrared laser field aligned with the molecular axis. We find dissociation probabilities of more than 60%, considerably higher than reported so far. We demonstrate that a full dimensional description of the electron dynamics is necessary to obtain accurate results for the combined ionization/dissociation dynamics.

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