Spin-Lattice Relaxation in Metal-Organic Platinum(II) Complexes

Details Spin-Lattice Relaxation in Metal-Organic Platinum(II) Complexes Spin-Lattice Relaxation in Metal-Organic Platinum(II) Complexes

1999-11-29

arxiv.org/abs/physics/9911076v1

Physics

Chemical Physics

9 pages, 3 figures (made from 4 .eps files), elsart.cls. Using dvips (dvipsk 5.58f), it may be necessary to manually edit the

Scientific paper

10.1016/S0009-2614(99)01298-1

The dynamics of spin-lattice relaxation (slr) of metal-organic Pt(II) compounds is studied. Often, such systems are characterized by pronounced zero-field splittings (zfs) of the lowest-lying triplets. Previous expressions for the Orbach slr process do not allow to treat such splitting patterns properly. We discuss the behavior of a modified Orbach expression for a model system and present results of a fit of the temperature dependence of the spin-lattice relaxation rate of Pt(2-thpy)$_2$ based on the modified expression.

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