Single-Shot Two Dimensional Time Resolved Coherent Anti Stokes Raman Scattering

Details Single-Shot Two Dimensional Time Resolved Coherent Anti Stokes Raman Scattering Single-Shot Two Dimensional Time Resolved Coherent Anti Stokes Raman Scattering

2006-12-06

arxiv.org/abs/physics/0612057v1

Physics

Optics

Scientific paper

10.1364/OE.15.001700

Single-shot time resolved Coherent Anti-Stokes Raman Scattering (CARS) is presented as a viable method for fast measurements of molecular spectra. The method is based on the short spatial extension of femtosecond pulses and maps time delays between pulses onto the region of intersection between broad beams. The image of the emitted CARS signal contains full temporal information on the field-free molecular dynamics, from which spectral information is extracted. The method is demonstrated on liquid samples of CHBr3 and CHCl3 and the Raman spectrum of the low-lying vibrational states of these molecules is measured.

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