Physics
Scientific paper
Dec 2003
adsabs.harvard.edu/cgi-bin/nph-data_query?bibcode=2003georl..30wsde2k&link_type=abstract
Geophysical Research Letters, Volume 30, Issue 23, pp. SDE 2-1, CiteID 2186, DOI 10.1029/2003GL018432
Physics
29
Atmospheric Composition And Structure: Biosphere/Atmosphere Interactions, Atmospheric Composition And Structure: Constituent Sources And Sinks, Atmospheric Composition And Structure: Troposphere-Composition And Chemistry
Scientific paper
Fluxes of biogenic volatile organic compounds (VOCs) were measured at a hardwood forest in northern Michigan (UMBS, Prophet research site) over the course of the growing and senescing season. Methanol, acetaldehyde, acetone and isoprene were found to be the most abundant biogenic VOCs with maximum fluxes (mixing ratios in ppbv) of 2.0 mg m-2 h-1 (21.0), 1.0 mg m-2 h-1 (2.7), 1.6 mg m-2 h-1 (5.6) and 7.6 mg m-2 h-1 (6), respectively. The emission patterns show distinct seasonal changes and indicate a spring peak for methanol due to rapid leaf expansion and a fall peak for acetone and acetaldehyde most likely attributed to senescing and decaying biomass; isoprene emissions peaked as expected in the summer. We estimate potential source strengths of 8.9 Tg (C) y-1 methanol, 2.7 Tg (C) y-1 acetaldehyde and 7.0 Tg (C) y-1 acetone for deciduous temperate forests, which is a substantial contribution to the global atmospheric VOC budget.
Fall Ray
Guenther Andreas
Hansel Armin
Karl Thomas
Spirig C.
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