Physics – Chemical Physics
Scientific paper
2010-10-04
Physics
Chemical Physics
5 pages, 5 figures
Scientific paper
The scattering and recombination processes between two triplet excitons in conjugated polymers are investigated by using a nonadiabatic evolution method, based on an extended Su-Schrieffer-Heeger model including interchain interactions. Due to the interchain coupling, the electron and/or hole in the two triplet excitons can exchange. The results show that the recombination induces the formation of singlet excitons, excited polarons and biexcitons. Moreover, we also find the yields of these products, which can contribute to the emission, increase with the interchain coupling strength, in good agreement with results from experiments.
An Zhenghua
Di Bangrang
Liu Xiao-Jing
Meng Yanling
Wang Ying-Dan
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