Scanning Near-Field Optical Coherent Spectroscopy of Single Molecules at 1.4 Kelvin

Details Scanning Near-Field Optical Coherent Spectroscopy of Single Molecules at 1.4 Kelvin Scanning Near-Field Optical Coherent Spectroscopy of Single Molecules at 1.4 Kelvin

2007-01-29

arxiv.org/abs/physics/0701321v1

Optics Letters, Vol. 32, Issue 11, pp. 1420-1422, 2007

Physics

Optics

3 pages, 5 figures, submitted to Optics Letters

Scientific paper

10.1364/OL.32.001420

We present scanning near-field extinction spectra of single molecules embedded in a solid matrix. By varying the molecule-tip separation, we modify the line shape of the spectra, demonstrating the coherent nature of the interaction between the incident laser light and the excited state of the molecule. We compare the measured data with the outcome of numerical calculations and find a very good agreement.

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