Quantum interference spectroscopy of RbHe exciplexes formed on helium nanodroplets

Details Quantum interference spectroscopy of RbHe exciplexes formed on helium nanodroplets Quantum interference spectroscopy of RbHe exciplexes formed on helium nanodroplets

2007-12-11

arxiv.org/abs/0712.1726v1

Phys. Rev. Lett. 100, 023401 (2008)

Physics

Atomic Physics

Scientific paper

10.1103/PhysRevLett.100.023401

Femtosecond multiphoton pump-probe photoionization is applied to helium nanodroplets doped with rubidium (Rb). The yield of Rb+ ions features pronounced quantum interference (QI) fringes demonstrating the coherence of a superposition of electronic states on a time scale of tens of picoseconds. Furthermore, we observe QI in the yield of formed RbHe exciplex molecules. The quantum interferogram allows to determine the vibrational structure of these unstable molecules. From a sliced Fourier analysis one can not only extract the population dynamics of vibrational states but also follow their energetic evolution during the RbHe formation.

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