Preparation and detection of states with simultaneous spin alignment and molecular orientation in PbO

Details Preparation and detection of states with simultaneous spin alignment and molecular orientation in PbO Preparation and detection of states with simultaneous spin alignment and molecular orientation in PbO

2008-07-30

arxiv.org/abs/0807.4851v1

Physics

Atomic Physics

Scientific paper

We are pursuing an experiment to measure the electric dipole moment of the electron using the molecule PbO. This measurement requires the ability to prepare quantum states with orientation of the molecular axis and, simultaneously, alignment of the electron spin perpendicular to this axis. It also requires efficient detection of the evolution of the spin alignment direction within such a state. We describe a series of experiments that have achieved these goals, and the features and limitations of the techniques. We also discuss possible new approaches for improved efficiency in this and similar systems.

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