Overlapping resonances in the control of intramolecular vibrational redistribution

Details Overlapping resonances in the control of intramolecular vibrational redistribution Overlapping resonances in the control of intramolecular vibrational redistribution

2007-03-28

arxiv.org/abs/quant-ph/0703263v1

J. Chem. Phys. 126, 124307 (2007)

Physics

Quantum Physics

10 pages, 7 figures

Scientific paper

10.1063/1.2710791

Coherent control of bound state processes via the interfering overlapping resonances scenario [Christopher et al., J. Chem. Phys. 123, 064313 (2006)] is developed to control intramolecular vibrational redistribution (IVR). The approach is applied to the flow of population between bonds in a model of chaotic OCS vibrational dynamics, showing the ability to significantly alter the extent and rate of IVR by varying quantum interference contributions.

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