Ortho-Para Conversion in CH3F. Self-Consistent Theoretical Model

Details Ortho-Para Conversion in CH3F. Self-Consistent Theoretical Model Ortho-Para Conversion in CH3F. Self-Consistent Theoretical Model

2000-03-21

arxiv.org/abs/physics/0003046v1

Appl. Magn. Reson. v.18, 363-374 (2000)

Physics

Chemical Physics

15 pages, 2 eps figures, REVTEX. Presented at the VI International Symposium on Magnetic Field and Spin Effects in Chemistry a

Scientific paper

A complete theoretical model of the nuclear spin conversion in 13CH3F induced by intramolecular ortho-para state mixing is proposed. The model contains parameters determined from the level-crossing spectra of the 13CH3F spin conversion. This set of parameters includes the ortho-para decoherence rate, the magnitude of the hyperfine spin-spin interaction between the molecular nuclei and the energy gap between the mixed ortho and para states. These parameters are found to be in a good agreement with their theoretical estimates.

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