Optical Stark Spectroscopy of the tilde{A}2Π- tilde{X}2Σ+ Band of BaOH

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Transitions of the tilde{A}2Π- tilde{X}2Σ+ band system of barium monohydroxide, BaOH, were observed and recorded from 11483-11485 Cm-1 and 12041-12044 Cm-1. The features were readily identified using the results of the Doppler-limited measurements. The laser induced fluorescence (LIF) spectrum was analyzed to give optimized field-free excited state parameters. The parameters for the tilde{X}2Σ+ state were constrained to the previously determined values. The permanent electric dipole moments for the tilde{X}2Σ+ and tilde{A}2Π states have been determined from the analysis of the optical Stark spectra for the R21(0.5), Q21(1.5), and R2(0.5) lines. The obtained values were μ(tilde{X}2Σ+)= 1.426(38)D and μ(tilde{A}2Π)= 0.477(7) D. The results are compared with predicted values from semi-empirical models and those for CaOH and SrOH.
J. G. Wang, J. D. Tandy and P. F. Bernath J. Mol. Spectrosc. 252, 31 (2008)
M. A. Anderson, M. D. Allen, W. L. Barclay, Jr, and L. M. Ziurys Chem. Phys. Lett 205, 415 (1993)
T. C. Steimle, D. A. Fletcher, K. Y. Jung and C. T. Scurlock J. Chem. Phys. 96, 2556 (1992).

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